Plasmon resonant amplification of a hot electron-driven photodiode
hot electrons, plasmonic resonance, plasmon, grating, photocurrent, non-equilibrium
ABSTRACT We report plasmon resonant excitation of hot electrons in a photodetector based on a metal/oxide/metal (Au/Al2O3/graphene) heterostructure. In this device, hot electrons, excited optically in the gold layer, jump over the oxide barrier and are injected into the graphene layer, producing a photocurrent. To amplify this process, the bottom gold electrode is patterned into a plasmon resonant grating structure with a pitch of 500 nm. The photocurrent produced in this device is measured using 633-nm-wavelength light as a function of incident angle. We observe the maximum photocurrent at ±10° from normal incidence under irradiation with light polarized parallel to the incident plane (p-polarization) and perpendicular to the lines on the grating, and a constant (angle-independent) photocurrent under irradiation with light polarized perpendicular to the incident plane (s-polarization) and parallel to the grating. These data show an amplification factor of 4.6× under resonant conditions. At the same angle (±10°), we also observe sharp dips in the photoreflectance corresponding to wavevector matching between the incident light and the plasmon mode in the grating. In addition, finite-difference time-domain simulations predict sharp dips in the photoreflectance at ±10°, and the electric field intensity profiles show clear excitation of a plasmon resonant mode when illuminated with p-polarized light at this angle.
Tsinghua University Press
Lang Shen,Nirakar Poudel,George N. Gibson,Bingya Hou,Jihan Chen,Haotian Shi,Ernest Guignon,William D. Page,Arturo Pilar,Stephen B. Cronin, Plasmon resonant amplification of a hot electron-driven photodiode. NanoRes.2018, 11(4): 2310–2314